A computational study of the transition from localized ignition to flame ball in lean hydrogen/air mixtures

Research output: Contribution to journalConference article

8 Citations (Scopus)

Abstract

A computational study has been conducted to determine the critical conditions for the transition from localized flame ignition and propagation to the establishment of a flame ball. Lean H2/air mixtures are investigated using a time-dependent, spherically symmetric code with detailed chemistry, transport, and radiation submodels. Results show that outwardly propagating spherical flames can be ignited for hydrogen mole fractions XH2 larger than ∼3.5%. Furthermore, assuming optically thin radiative heat loss, flame balls can be established from centrally ignited premixed spherical flames only within a narrow range of mixture compositions (i.e., ∼3.5% < XH2 < ∼6.5%). For ∼6.5% < XH2 ∼11%, flames propagate until radiative extinction, never evolving into flame balls, while for XH2 > ∼11%, the expanding spherical flames develop asymptotically into planar propagating flames. These findings corroborate the experimental result that the range of mixtures within which flame balls have been observed is much narrower than that predicted by previous one-dimensional instability analysis of the flame ball, where it was shown that steady flame balls exist for 3.5% < XH2 < 10.7%. The present simulation also shows that the dynamic transition from a spherically propagating flame to the flame ball controls the range of mixtures for which flame balls can be reached, with radiative loss being both the requisite mechanism for and the limiting mechanism against the dynamic transformation. Additional calculations show that the size of the flame ball is noticeably enlarged when radiative reabsorption is incorporated.

Original languageEnglish (US)
Pages (from-to)1917-1924
Number of pages8
JournalProceedings of the Combustion Institute
Volume28
Issue number2
DOIs
StatePublished - Jan 1 2000
Event30th International Symposium on Combustion - Chicago, IL, United States
Duration: Jul 25 2004Jul 30 2004

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ignition
Ignition
balls
Hydrogen
flames
air
hydrogen
Air
Heat losses
Radiation
Chemical analysis
chemistry

Cite this

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title = "A computational study of the transition from localized ignition to flame ball in lean hydrogen/air mixtures",
abstract = "A computational study has been conducted to determine the critical conditions for the transition from localized flame ignition and propagation to the establishment of a flame ball. Lean H2/air mixtures are investigated using a time-dependent, spherically symmetric code with detailed chemistry, transport, and radiation submodels. Results show that outwardly propagating spherical flames can be ignited for hydrogen mole fractions XH2 larger than ∼3.5{\%}. Furthermore, assuming optically thin radiative heat loss, flame balls can be established from centrally ignited premixed spherical flames only within a narrow range of mixture compositions (i.e., ∼3.5{\%} < XH2 < ∼6.5{\%}). For ∼6.5{\%} < XH2 ∼11{\%}, flames propagate until radiative extinction, never evolving into flame balls, while for XH2 > ∼11{\%}, the expanding spherical flames develop asymptotically into planar propagating flames. These findings corroborate the experimental result that the range of mixtures within which flame balls have been observed is much narrower than that predicted by previous one-dimensional instability analysis of the flame ball, where it was shown that steady flame balls exist for 3.5{\%} < XH2 < 10.7{\%}. The present simulation also shows that the dynamic transition from a spherically propagating flame to the flame ball controls the range of mixtures for which flame balls can be reached, with radiative loss being both the requisite mechanism for and the limiting mechanism against the dynamic transformation. Additional calculations show that the size of the flame ball is noticeably enlarged when radiative reabsorption is incorporated.",
author = "Stephen Tse and L. He and Law, {C. K.}",
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A computational study of the transition from localized ignition to flame ball in lean hydrogen/air mixtures. / Tse, Stephen; He, L.; Law, C. K.

In: Proceedings of the Combustion Institute, Vol. 28, No. 2, 01.01.2000, p. 1917-1924.

Research output: Contribution to journalConference article

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N2 - A computational study has been conducted to determine the critical conditions for the transition from localized flame ignition and propagation to the establishment of a flame ball. Lean H2/air mixtures are investigated using a time-dependent, spherically symmetric code with detailed chemistry, transport, and radiation submodels. Results show that outwardly propagating spherical flames can be ignited for hydrogen mole fractions XH2 larger than ∼3.5%. Furthermore, assuming optically thin radiative heat loss, flame balls can be established from centrally ignited premixed spherical flames only within a narrow range of mixture compositions (i.e., ∼3.5% < XH2 < ∼6.5%). For ∼6.5% < XH2 ∼11%, flames propagate until radiative extinction, never evolving into flame balls, while for XH2 > ∼11%, the expanding spherical flames develop asymptotically into planar propagating flames. These findings corroborate the experimental result that the range of mixtures within which flame balls have been observed is much narrower than that predicted by previous one-dimensional instability analysis of the flame ball, where it was shown that steady flame balls exist for 3.5% < XH2 < 10.7%. The present simulation also shows that the dynamic transition from a spherically propagating flame to the flame ball controls the range of mixtures for which flame balls can be reached, with radiative loss being both the requisite mechanism for and the limiting mechanism against the dynamic transformation. Additional calculations show that the size of the flame ball is noticeably enlarged when radiative reabsorption is incorporated.

AB - A computational study has been conducted to determine the critical conditions for the transition from localized flame ignition and propagation to the establishment of a flame ball. Lean H2/air mixtures are investigated using a time-dependent, spherically symmetric code with detailed chemistry, transport, and radiation submodels. Results show that outwardly propagating spherical flames can be ignited for hydrogen mole fractions XH2 larger than ∼3.5%. Furthermore, assuming optically thin radiative heat loss, flame balls can be established from centrally ignited premixed spherical flames only within a narrow range of mixture compositions (i.e., ∼3.5% < XH2 < ∼6.5%). For ∼6.5% < XH2 ∼11%, flames propagate until radiative extinction, never evolving into flame balls, while for XH2 > ∼11%, the expanding spherical flames develop asymptotically into planar propagating flames. These findings corroborate the experimental result that the range of mixtures within which flame balls have been observed is much narrower than that predicted by previous one-dimensional instability analysis of the flame ball, where it was shown that steady flame balls exist for 3.5% < XH2 < 10.7%. The present simulation also shows that the dynamic transition from a spherically propagating flame to the flame ball controls the range of mixtures for which flame balls can be reached, with radiative loss being both the requisite mechanism for and the limiting mechanism against the dynamic transformation. Additional calculations show that the size of the flame ball is noticeably enlarged when radiative reabsorption is incorporated.

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