An elegant post-growth process science protocol to improve the material properties of complex oxide thin films for tunable device applications

M. W. Cole, R. C. Toonen, S. G. Hirsch, M. Ivill, E. Ngo, C. Hubbard, S. Ramanathan, A. Podpirka

Research output: Contribution to journalConference articlepeer-review

Abstract

We report on an innovative isothermal post-growth/crystallization process that utilizes ultraviolet (UV)-photon irradiation. We fabricated Ba1-xSrxTiO3 (BST) thin films using metalorganic solution deposition (MOSD) and UV-photon irradiation isothermal treatment via two protocols: in situ crystallized UV-photon irradiated films, and post-crystallization UV-photon irradiated films. Isothermal UV-photon irradiation treatment improves the structural quality of the BST films, and the irradiated films possessed lattice parameters close to the bulk values, which is evidence for a reduction in oxygen vacancies. MOSD fabricated BST films crystallized via conventionally furnace annealing and subsequently exposed to UV-photon irradiation possessed improved structural, dielectric, and electrical quality.

Original languageAmerican English
Pages (from-to)34-46
Number of pages13
JournalIntegrated Ferroelectrics
Volume126
Issue number1
DOIs
StatePublished - 2011
Externally publishedYes
EventSymposium on Ferroelectric and Piezoelectric Materials, Devices, and Applications - 19th International Materials Research Congress, IMRC 2010 - Cancun, Mexico
Duration: Aug 15 2010Aug 19 2010

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Control and Systems Engineering
  • Ceramics and Composites
  • Condensed Matter Physics
  • Electrical and Electronic Engineering
  • Materials Chemistry

Keywords

  • BST
  • UV-photon irradiation
  • dielectric loss
  • material property balance
  • microwave devices
  • phase shifter
  • thin film processing

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