Field dependent carrier transport mechanisms in metal-insulator-metal devices with Ba0.8Sr0.2TiO3/ZrO2 heterostructured thin films as the dielectric

Santosh K. Sahoo, H. Bakhru, Sumit Kumar, D. Misra, Colin A. Wolden, Y. N. Mohapatra, D. C. Agrawal

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Abstract

Ba0.8Sr0.2TiO3/ZrO2 heterostructured thin films with different individual layer ZrO 2thicknesses are deposited on Pt/Ti/SiO2/Si substrates by a sol-gel process. The current versus voltage (I-V) measurements of the above multilayered thin films in metal-insulator-metal (MIM) device structures are taken in the temperature range of 310 to 410K. The electrical conduction mechanisms contributing to the leakage current at different field regions have been studied in this work. Various models are used to know the different conduction mechanisms responsible for the leakage current in these devices. It is observed that Poole-Frenkel mechanism is the dominant conduction process in the high field region with deep electron trap energy levels (φ) whereas space charge limited current (SCLC) mechanism is contributing to the leakage current in the medium field region with shallow electron trap levels (E t). Also, it is seen that Ohmic conduction process is the dominant mechanism in the low field region having activation energy (Ea) for the electrons. The estimated trap level energy varies from 0.2 to 1.31 eV for deep level traps and from 0.08 to 0.18 eV for shallow level traps whereas the activation energy for electrons in ohmic conduction process varies from 0.05 to 0.17 eV with the increase of ZrO2 sub layer thickness. An energy band diagram is given to explain the dominance of the various leakage mechanisms in different field regions for these heterostructured thin films.

Original languageEnglish (US)
Title of host publicationSolution Synthesis of Inorganic Functional Materials - Films, Nanoparticles, and Nanocomposites
Pages53-60
Number of pages8
DOIs
StatePublished - Dec 13 2013
Event2013 MRS Spring Meeting - San Francisco, CA, United States
Duration: Apr 1 2013Apr 5 2013

Publication series

NameMaterials Research Society Symposium Proceedings
Volume1547

Other

Other2013 MRS Spring Meeting
CountryUnited States
CitySan Francisco, CA
Period4/1/134/5/13

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All Science Journal Classification (ASJC) codes

  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering
  • Materials Science(all)

Cite this

Sahoo, S. K., Bakhru, H., Kumar, S., Misra, D., Wolden, C. A., Mohapatra, Y. N., & Agrawal, D. C. (2013). Field dependent carrier transport mechanisms in metal-insulator-metal devices with Ba0.8Sr0.2TiO3/ZrO2 heterostructured thin films as the dielectric. In Solution Synthesis of Inorganic Functional Materials - Films, Nanoparticles, and Nanocomposites (pp. 53-60). (Materials Research Society Symposium Proceedings; Vol. 1547). https://doi.org/10.1557/opl.2013.85S