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Outlook for active plasma spectroscopy with entangled two-photon absorption

  • David R. Smith
  • , Nivedan Vishwanath
  • , Michael Zepp
  • , Matthias Beuting
  • , Daniel J.Den Hartog
  • , Benedikt Geiger
  • , Scott T. Sanders
  • , Xuting Yang
  • , Jennifer T. Choy

Research output: Contribution to journal › Article › peer-review

Abstract

Entangled two-photon absorption (ETPA) exhibits a quantum-enhanced two-photon absorption cross-section and a linear scaling with incident power that exceeds classical two-photon absorption (TPA) at low photon flux. Here, we assess the feasibility and applications of ETPA for active plasma spectroscopy. The ETPA-absorbed power for an Ar+ species in a helicon plasma scenario is calculated to be as high as 0.6 nW cm−1 along the incident beam path for nondegenerate-entangled photon pairs that are near-resonant with an intermediate level. The ETPA absorption power exceeds classical TPA and Bremsstrahlung emission, a necessary condition for a feasible fluorescence measurement. Applications of ETPA plasma spectroscopy may include trace impurity detection, ground-state excitation, and continuous-wave pumping for high-bandwidth turbulence measurements. Possible benefits of plasma measurements are less harm to optical components with lower incident flux and reduced stray light that can contaminate optical diagnostics.

Original languageEnglish (US)
Article number505204
JournalJournal of Physics D: Applied Physics
Volume58
Issue number50
DOIs
StatePublished - Dec 15 2025
Externally publishedYes

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics
  • Acoustics and Ultrasonics
  • Surfaces, Coatings and Films

Keywords

  • active plasma spectroscopy
  • entangled two photon absorption
  • laser-aided plasma diagnostics

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